Example 1
Cs3Cr2Br9 provides an example of a three dimensional interacting spin-dimer system (s=3/2) where the ground state (G.S.) is an S = 0 singlet state and the first excited state, an S = 1 triplet, is separated from the G.S. by an energy gap Δ≈0.2 meV. In a magnetic field, because of the Zeeman splitting of the S = 1 state, a phase transition occurs at a critical field Hc1, when the lowest gap closes.Above Hc1, the field-induced magnetic ordering is due to the inter-dimer couplings. Figure 1 shows the field dependence of the three energy gaps. Contrary to TlCuCl3, no Bose-remains gapped in the field-induced ordered phase. This is probably related to the sizable single-ion anisotropy.